Tunable fractal shapes in self-avoiding polygons and planar vesicles

Abstract
The shapes of self-avoiding continuum and lattice polygons of N monomers in a plane are studied using Monte Carlo simulations and exact enumeration. To model vesicles, a pressure increment Δp=pin-pout, is included. For N≫1 and Δp=0, the usual universal fractal shapes appear; but for Δp≠0, continuously variable fractal shapes are found controlled by the variable x∝ΔpN2ν where ν=1/DF=3/4. Thus, the ratio of principal radii of gyration Σ(x)=〈RG,min2〉/〈RG,max2〉 changes smoothly from Σ(+∞)=1, for circles, through Σ(0)≃0.39, to Σ(-∞)≃0.23, which corresponds to branched polymers.

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