Abstract
Reduction (NaBH4) of adamantanethione gives high yields of pure 2-adamantanethiol, from which several derivatives including the methyl sulfide, sulfoxide, and sulfone were prepared. The sulfenyl chloride was prepared and used insitu. From the n.m.r. spectra the aromatic solvent-induced shifts Δ = τ(benzene) – τ(CCl4 or CDCl3) were determined, where possible.

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