Abstract
The line intensities in Raman spectra of molecules are determined by means of a perturbation calculation. For this purpose the vibrating molecule was considered under the conditions of static electric fields causing the perturbation in directions parallel to the axis of a Cartesian co-ordinate system of the molecule. The calculated perturbation terms are inserted into the Hartree-Fock - Operator used in the CNDO/II-theory6. This calculation yields the induced dipole moment as a function of the normal coordinate Q, from which the polarizability change upon Q is obtained.

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