Substitution on five µ-oxo/µ-sulphido incomplete cuboidal MoIV3ions [Mo3OxS4–x(H2O)9]4+: kinetic effects resulting from the replacement of core oxo by sulphido ligands

Abstract
A 570-fold spread in rate constants (25 °C), [H+]= 2.0 M, is observed for 1 : 1 NCS substitution (of H2O) at Mo on the title complexes, with replacement of core µ3(O) by µ3(S) decreasing (factor of 10), and further replacement of the three µ2(O) by µ2(S) increasing (factor of 570) the rate of substitution.
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