The solution of the Schrödinger equation by the (t,t) method using the wave operator procedure: Theory and application to molecular photodissociation with ultrashort laser pulses

Publisher Website
Google Scholar
Abstract
A new method for studying intense field photodissociation of molecules using ultrashort laser pulses is presented. The method is based on a generalized Floquet approach making use of the (t,t) formalism and the wave operator theory. The usefulness of the scheme for ultrafast photodissociation is illustrated by studying H2+ multiphoton dissociation with moderately intense and very short laser pulses.