The molecular orbital theory of chemical valency VII. Molecular structure in terms of equivalent orbitals
- 22 February 1951
- journal article
- Published by The Royal Society in Proceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences
- Vol. 205 (1082) , 357-374
- https://doi.org/10.1098/rspa.1951.0034
Abstract
The twofold method of describing molecular structure, developed in earlier parts, is applied to a number of simple molecules in order to elucidate various properties of chemical interest. The molecules, methane, ammonia, water and hydrogen fluoride, are used to illustrate the properties of lone pairs of electrons and to show the significance of tetrahedral orbitals. Ethylene provides an example of the dual way of describing a double bond, either as a σ bond and a π bond, or as two equivalent bonds. The triple bonds of acetylene and nitrogen are similarly discussed, and an answer sought to the question why the lone pair of electrons on each atom of the nitrogen molecule differ from that of ammonia. Butadiene and benzene are considered as examples of conjugated systems in order to bring out the unlocalized character of the equivalent orbitals used to describe them, thus illustrating an essential difference between saturated and unsaturated molecules. There is also a short discussion of the boron hydrides and cyclopropane, each of which present some unusual features.Keywords
This publication has 12 references indexed in Scilit:
- An Electrical Apparatus for Herpetological CollectingIchthyology & Herpetology, 1950
- The molecular orbital theory of chemical valency. IV. The significance of equivalent orbitalsProceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences, 1950
- Sounds Produced by the Suwannee TerrapinIchthyology & Herpetology, 1950
- The Structure of Diborane and Related Molecules.Chemical Reviews, 1947
- The properties of bonds involving carbonDiscussions of the Faraday Society, 1947
- Electron Deficient Molecules. I. The Principles of Hydroboron StructuresJournal of the American Chemical Society, 1945
- Molecular electronic spectra, dispersion and polarization: The theoretical interpretation and computation of oscillator strengths and intensitiesReports on Progress in Physics, 1941
- Zur Frage der chemischen BindungThe European Physical Journal A, 1932
- THE NATURE OF THE CHEMICAL BOND. APPLICATION OF RESULTS OBTAINED FROM THE QUANTUM MECHANICS AND FROM A THEORY OF PARAMAGNETIC SUSCEPTIBILITY TO THE STRUCTURE OF MOLECULESJournal of the American Chemical Society, 1931
- Directed Valence in Polyatomic MoleculesPhysical Review B, 1931