Biosynthesis of collectodiol and related polyketide macrodiolides in Cytospora sp. ATTCC 20502: synthesis and metabolism of advanced intermediates

Abstract
The triene 3 and 6 have been syntesised in specifically labeled from and their incorporation into the macrodiolide, colletodio 1 demonstrated in cultures of Cytospora sp. ATCC 20502; results of a biomimetic reaction indicate that both colletoketol 2 and grahamimycin A17 may be biosynthesized in a single oxidation step from collectodiol.

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