Coherence transfer in the rotating frame

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Abstract
Coherence transfer between heteronuclear spin species in the rotating frame is analysed in view of application to heteronuclear two-dimensional cross-correlation spectroscopy in liquids. The general formalism and applications to simple spin systems are presented. In particular, the longitudinal and transverse coherence transfer functions are evaluated and discussed in terms of transfer efficiency, oscillation frequencies, phase anomalies and multiplet effects.