Ab initioHartree-Fock calculation of the force constants and geometry of HNF2and H2NF

Abstract
Force constants have been calculated for H2NF and HNF2 from ab initio Hartree-Fock wavefunctions by the force method, using 7s3p/1 gaussian basis sets. The force field of HNF2, obtained from a combination of the theoretical results with the experimental frequencies, can be considered as the most reliable one at present. Previous force fields are discussed critically. From a full optimization the predicted geometry of H2NF is: NF = 1·399 Å, NH = 1·018 Å, HNF = 102·9° and HNH = 105·9°.

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