Time dependence of photon correlations in a three-level atomic cascade

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Abstract
The question of the temporal correlation of photons arising from a three-level atomic cascade is considered by calculating the joint probability of photoelectric detection for two detectors placed in the far field of the atomic emission. The analysis is carried out in the Heisenberg picture and involves the use of dipole, adiabatic (Weisskopf-Wigner), and rotating-wave approximations. Except for a small interval about zero time delay, which is however too short to be detected, it is found that the temporal correlation between emitted photons is one of sequential but otherwise statistically independent events, even when Landau’s generalized decay and frequency-shift terms are included. This result is compared with a well-known expression for the joint spectral density of the emitted photons.

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