Reversible oxygenation of metal complexes: electronic and steric factors

Abstract
The rates of oxygen addition to trans-[IrCl(CO)-(R3P)2](R3P = tertiary phosphine) and the stability of the resulting dioxygen adducts, [O2IrCl(CO)(R3P)2], increase with increasing basicity of the substituent R, provided the substituents have comparable structures; the geometry of R exerts a profound effect on the dynamics of these reactions.

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