Optical determination of the antiferromagnetic exchange constant between nearest-neighbor ions in Te
- 15 October 1985
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 32 (8) , 5132-5137
- https://doi.org/10.1103/physrevb.32.5132
Abstract
Optical splittings of the band-edge exciton in Te have been measured at 1.45 K with dc magnetic fields B up to 20 T, using magnetoreflectance in the Faraday configuration. The splitting Δ between the highest- and lowest-energy components, involving ±(3/2) hole states, follows a modified Brillouin function at low values of B. At higher values of B, Δ exhibits temperature-broadened, steplike increases due to the magnetic-field-induced alignment of the antiferromagnetically coupled nearest-neighbor (NN) -ion pairs. The first of the expected five steps was observed at =11.5±0.5 T, which yields a value K for the nearest-neighbor antiferromagnetic exchange constant. The presence of a second step is indicated at =19.5±1.0 T, somewhat below the predicted value of 2.
Keywords
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