Dynamics of stochastic systems in nonlinear optics. I. General formalism

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Abstract
Stochastic theories have been used for a long time to describe relaxation as well as line-shape functions. Since the pioneering work of Kubo, these theories have gained considerable interest in the application to optical processes. While previous theories focused on stochastic descriptions of the relaxation, our emphasis is on the dynamics induced by stochastic interactions in a system undergoing relaxation and dephasing processes, including pure dephasing. All the theories based either on the Hilbert-space representation, or on the Liouvillian-space representation, but requiring spectral decomposition methods, are unable to describe these effects simultaneously. In this paper, the implications of the statistical properties of the stochastic variables on the dynamics are elucidated, and the general time evolution of a stochastic N-level system is established in the particular Markovian or weakly colored noise cases.

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