Magnetodielectric Effects from Spin Fluctuations in Isostructural Ferromagnetic and Antiferromagnetic Systems

We report on the effects of spin fluctuations, magnetic ordering, and external magnetic field on the dielectric constant of the ferromagnet ${\mathrm{S}\mathrm{e}\mathrm{C}\mathrm{u}\mathrm{O}}_3$, and the antiferromagnet ${\mathrm{T}\mathrm{e}\mathrm{C}\mathrm{u}\mathrm{O}}_3$. A model based on the coupling between uniform polarization and the $q$-dependent spin-spin correlation function is presented to explain the different behaviors for these isostructural compounds. The large magnetocapacitance near the transition temperature in the ferromagnet ${\mathrm{S}\mathrm{e}\mathrm{C}\mathrm{u}\mathrm{O}}_3$ suggests routes to enhancing the magnetodielectric response for practical applications.