Abstract
Experimental measurements of ultraviolet and visible emission from two samples containing 233U suggest the deexcitation of a reported 3.5 eV isomeric level in 229Th. The unique phenomenon of ultraviolet γ-ray emission was observed from this level. Results are consistent with theoretical arguments suggesting that the nucleus can also deexcite via an inelastic electronic bridge mechanism. These observations indicate the exotic phenomenon of nuclear emission in the optical band, and open new areas of physics related to nuclear-atomic interaction.