Abstract
The reaction of tricarbonyl(4-methoxy-1-methylcyclohexadienyl)iron hexafluorophosphate (1), or tricarbonyl(2–8a-η-3-methoxyhexahydronaphthyl)iron tetrafluoroborate (5) with cyanide anion results in addition of the nucleophile to the more electron-deficient terminus of the dienyl system, forming quaternary centres and angularly substituted compounds (2) and (6), respectively.

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