Pure vibrational Raman spectra of simple molecular crystals: Ar–N2, Ar–O2, Ar–CO, β–CO

Abstract
Interferometric techniques have been employed to study the polarized (pure) vibrational Raman spectra of N2, O2, and CO as dilute solutions in single crystal matrices of Ar. The observation of a clearly resolved and concentration dependent spectral structure is interpreted as arising from the clustering of solute molecules.

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