Two-dimensional band structure and self-energy of Bi(111) near theΓ¯point

Abstract
Angle-resolved photoemission spectroscopy with synchrotron radiation was used to map the Fermi surface and the dispersion of the associated bands of Bi(111) near the Γ¯ point. Using variable photon energies we prove the two-dimensional nature of these bands. From fits of the spectral function A(ω,k) to momentum distribution curves of the hole band we determined the imaginary part of the electron self-energy ImΣ(ω). The small energy dependence of ImΣ(ω) near the Fermi level, which can be explained by electron-phonon interactions, indicates nonquasiparticle behavior. By means of a Hilbert transform of ImΣ(ω) we extract the energy dependence of ReΣ(ω). Based on the bulk Debye phonon model we determine the electron-phonon coupling constant λ=0.6±0.05