Laser-Induced Interference, Focusing, and Diffraction of Rescattering Molecular Photoelectrons
- 23 November 2004
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 93 (22) , 223003
- https://doi.org/10.1103/physrevlett.93.223003
Abstract
We solve the time-dependent Schrödinger equation in three dimensions for in a one-cycle laser pulse of moderate intensity. We consider fixed nuclear positions and Coulomb electron-nuclear interaction potentials. We analyze the field-induced electron interference and diffraction patterns. To extract the ionization dynamics we subtract the excitations to low-lying bound states explicitly. We follow the time evolution of a well-defined wave packet that is formed near the first peak of the laser field. We observe the fragmentation of the wave packet due to molecular focusing. We show how to retrieve a diffraction molecular image by taking the ratio of the momentum distributions in the two lateral directions. The positions of the diffraction peaks are well described by the classical double slit diffraction rule.
Keywords
This publication has 33 references indexed in Scilit:
- Reading diffraction images in strong field ionization of diatomic moleculesJournal of Physics B: Atomic, Molecular and Optical Physics, 2004
- Two-pulse alignment of moleculesJournal of Physics B: Atomic, Molecular and Optical Physics, 2004
- Time-Resolved Double Ionization with Few Cycle Laser PulsesPhysical Review Letters, 2003
- Electron diffraction in above-threshold ionization of moleculesPhysical Review A, 2002
- Experimental Observation of Revival Structures in Picosecond Laser-Induced Alignment of I2Physical Review Letters, 2001
- Correlated multiphoton double ionization of helium: The role of nonadiabatic tunneling and singlet recollisionPhysical Review A, 2001
- Erratum: Physics of correlated double ionization of atoms in intense laser fields: Quasistatic tunneling limit [Phys. Rev. A63, 033404 (2001)]Physical Review A, 2001
- Few Cycle Dynamics of Multiphoton Double IonizationPhysical Review Letters, 2001
- Molecular dynamics and time reversibilityJournal of Statistical Physics, 1993
- A space‐saving modification of Davidson's eigenvector algorithmJournal of Computational Chemistry, 1990