The antiferromagnetic form factor of La2NiO4

Abstract
Neutron‐diffraction techniques have been used to study the antiferromagnetic form factor of a La2NiO4 single crystal at 15 K. The antiferromagnetic form factor was obtained by measuring the integrated intensities of 16 magnetic reflections. A plateau is clearly seen at low Q (up to 3 Å−1) in the experimentally determined form factor, similar to those observed for La2CuO4 and Sr2CuO2Cl2. As in the case of these latter compounds, the fit of the experimental data by a Ni2+ ionic form factor is not satisfactory. The experimental data are compared with a recent spin‐polarized band calculation and with a covalency model.