Raman study of CF4 in liquid Ar

Abstract
The rotational behaviour of CF4 dissolved in liquid argon is derived from the band contour analysis of Raman spectra recorded over the concentration range from 10-2 mole fraction to 1 mole fraction at 85 K. The angular momentum correlation times have been determined with the help of the J-diffusion model and used to apply the rough hard sphere model. A study of the transition dipole-transition dipole (TD-TD) interaction is made using the v 3 mode at 85 K for different concentrations.