Hopping conduction in thin films of tetrathiotetracene

Abstract
Measurements of the AC and DC conductivity of vacuum-deposited thin films of tetrathiotetracene are described. Long-range potential wells associated with TTT-oxygen complexes play a dominant role in the transport process. In particular DC conduction requires movement between these wells while AC conduction occurs between sites within the wells. A density of states of approximately 1019cm-3 calculated from the AC data is in agreement with the density of carriers determined from an electron spin resonance study. High-field measurements are analysed in terms of a Poole-Frenkel effect, which gives a barrier height of 0.26 eV compared to a DC activation energy of 0.28 eV.

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