Transport of excitations in disordered systems: Self-consistent density resummation
- 15 October 1984
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 30 (8) , 4426-4440
- https://doi.org/10.1103/physrevb.30.4426
Abstract
New self-consistent equations for the transport of excitations in disordered systems are derived based on a resummation procedure of the density expansion. Both local-time [partial-time-ordering prescription (POP)] and convolution-type [chronological-time-ordering prescription] equations are explored. Application is made to a system consisting of a random mixture of donors and traps with a general type of transfer rate . We calculate the probability of remaining in the original site as well as the second moment of the distribution of excitations . The POP equations reduce to the exact Forster solution for in the case of traps only. We analyze the long-time behavior of and its dependence on . We find a percolation-type transition when has a cutoff [i.e., for ] but in all other cases the system is diffusive at long times [ vanishes and diverges linearly in time].
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