Synthesis of (±)-[6]-gingerol (pungent principle of ginger) and relatives via directed aldol reactions

Abstract
Selective deprotonation of trimethylsilyl zingerone (2: R = Me3Si) and trimethylsilylvanillylacetone (7:R = Me3Si) can be effected; the resulting anions condense readily with aldehydes and acylimidazoles to provide short syntheses of the ginger root constituents (±)-[4]-, (±)-[6]-(an organoleptic principle), (±)-[10]-gingerol, and di-O-methylhexahydrocurcumin, and the related dehydro-[6]-gingerol and [6]-gingerdione.

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