Angular distributions and branching ratios of the electrons ejected from the Ba [6p1/2(3/2)ns1/2]J=1 autoionizing states

Abstract
We describe the first comprehensive measurements of the energy distribution, branching ratios, and angular distributions of electrons ejected from Ba i [6p1/2 ns1/2(3/2) ]J=1 states in their autoionization to the Ba ii 6s, 5d, and 6p ion states. These measurements are made using a stepwise laser excitation scheme, which results in excitation of only the bound part of the autoionizing states. Furthermore, the laser excitation of these autoionizing states through the spherically symmetric Ba i 6sns 1 S0 intermediate states results in simplified electron angular distributions. We find that the Ba i [6p1/2 ns1/2(3/2) ]J=1 states autoionize predominantly to an excited state of the Ba+ ion. The interaction between the Ba i [6p1/2 ns1/2 ]J=1 and the Ba i [6p3/2 ns1/2 ]J=1 series manifests itself in the sharp variation in the electron asymmetry parameter β near the neighborhood of the interaction. We also present a simple analysis of our results incorporating the multichannel quantum-defect theory.