Quantitative trace element determination in thin samples by total reflection x‐ray fluorescence using the scattered radiation method

Abstract
It is shown that samples exposed under total reflection conditions obey the relationship Ii/Iinc = KCi, where Ii is the x‐ray fluorescence intensity due to element i of concentration Ci, Iinc is the intensity of the scattered incoherent radiation and K is a constant. An experiment on the determination of sulphur in diesel fuel confirmed this derivation. This relationship affords a simple and fast method for quantitative trace element determination, requiring virtually no sample preparation and extremely small amounts (<Iμl). Other advantages include its insensitivity to instrumental variations and changes in excitation conditions or in sample characteristics such as particle size and sample amount.

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