Metal-insulator transition in layered manganites: (La1zNdz)1.2Sr1.8Mn2O7

Abstract
Lattice effects on the anisotropic magnetic and transport properties have been investigated for single crystals of (La1zNdz)1.2Sr1.8Mn2O7 with a layered structure. The ferromagnetic transition temperature TC is suppressed from TC=130 K for z=0.0 to 80 K for z=0.2, and eventually the transition disappears beyond z=0.4. From the significant change of the magnetic anisotropy, we have found that the suppression originates from the increasing d3z2r2 character in the occupied eg state due to the Jahn-Teller distortion of the MnO6 octahedra. Our observations indicate that the effects of chemical substitution are qualitatively different between the cubic and layered doped manganites.