Organometallic vapor-phase epitaxial growth and characterization of the metastable alloy InP1−xSbx

Abstract
The III‐V metastable alloy InP1−x Sbx has been grown for the first time with compositions well inside the miscibility gap. Despite the large miscibility gap at the growth temperatures of 480–600 °C, epilayers with compositions covering the entire range from x=0 to 1.0 have been grown successfully by organometallic vapor‐phase epitaxy at atmospheric pressure using the reactants trimethylindium, trimethylantimony, and phosphine. The 10‐K energy band gap as a function of composition was determined from photoluminescence measurements combined with x‐ray diffraction and electron microprobe analysis. The bowing parameter for the band‐gap energy of the InP1−x Sbx was estimated to be 1.9±0.1 eV. The lattice dynamics have been studied using Raman spectroscopy in the frequency range from 150 to 400 cm1. Long wavelength optical phonons display a ‘‘two‐mode’’ behavior throughout the entire composition range. The InP‐like longitudinal‐optical and transverse‐optical modes shift to lower frequency with increasing Sb concentration.

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