Über die Pyrolyse von Pent‐1‐en‐3,3‐d2

Abstract
On the Pyrolysis of Pent‐1‐ene‐3,3‐d2The distribution of deuterium in the main products of the thermal decomposition of pent‐1‐ene‐3,3‐d2 at 550 to 650°C was studied and interpreted. The results include conclusions on kinetic isotope effects, on relative reactivities of different CH‐bonds, and on the importance of nonterminal radical addition. It is shown that butadiene‐d2 detected in the isotopically labeled butadiene fraction is a reliable target molecule for the homoallylic rearrangement of the pent‐1‐ene‐4‐yl‐3,3‐d2 radical.

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