Track formation inSiO2quartz and the thermal-spike mechanism

Abstract
α-quartz has been irradiated with heavy ions: F19, S32, and Cu63 at an energy of about 1 MeV/amu in order to cover a range of electronic stopping powers dE/dx between 2.4 and 9 keV/nm and Ni58, Kr86, Te128, Xe129, Ta181, and Pb208 between 1 and 5.8 MeV/amu for dE/dx>7 keV/nm. The extent of the induced damage is determined using Rutherford backscattering ion channeling with a 2-MeV He4 beam. The damage cross section A is obtained using a Poisson law Fd=1-exp(-Aφt), where φ is the flux and t the irradiation time. This damage cross section is linked to the effective radius Re through the relation ARe2, where Re is the radius of an equivalent cylinder of damage. Using high-resolution electron microscopy, cylinders of amorphous matter have been observed, whose radius corresponds to Re when the track is continuous (i.e., for A≥1.3×1013 cm2; Re≥2 nm). A thermal-spike model is applied to calculate the radii of the observed tracks assuming that the observed amorphous cylinders correspond to a rapid quench of a molten liquid phase along the ion path. The model is applied only when the latent track is continuous and cylindrical. A good agreement is obtained taking into account that the initial spatial energy deposition on the electrons depends on the ion velocity.