Fragment mass and kinetic energy distributions forPu242(sf),Pu241(nth,f), andPu242(γ,f)

Abstract
Energy correlation measurements were performed for the spontaneous fission of Pu242, the thermal-neutron-induced fission of Pu241, and the photofission of Pu242 with 12-, 15-, 20-, and 30- MeV bremsstrahlung. The photofission cross section for Pu242 was determined up to 30 MeV. For Pu242(sf) the overall kinetic energy distribution is strongly asymmetric and the overall mass distribution has a very high peak yield (9%). Important deviations of the average total kinetic energy release Ek* and the average light and heavy fragment masses mL* and mH* from the systematics of Unik et al. are also observed for this fissioning system. These effects can be explained in the framework of the static scission point model by the strong preferential formation of a shell-stabilized scission configuration with the neutron number of the heavy and light fragments in the vicinity of the spherical N=82 neutron shell and the deformed N=66 neutron shell, respectively. A decrease of Ek* with the average excitation energy Eexc(Ee), dEk*dEexc(Ee)=0.30±0.04, is observed in the photofission of Pu242. A study of the energy-mass correlations shows that the mentioned decrease is caused predominantly by a diminution of the shell corrections in the mass region of the spherical N=82 neutron shell. A comparison of the mass and kinetic energy distributions obtained in this work for Pu242, with previously reported results for Pu240 and Pu244 and with scission point model calculations, is also included.