Abstract
Using a surface-ionization mass spectrometer, the natural U238/U235 abundance ratio in uranium obtained from Great Bear Lake Pitchblende has been measured to be 137.80 ± 0.14. From a survey of results reported in the literature on U234 a best value of 17,325 ± 550 was estimated for the natural U238/U234 abundance ratio. The corresponding isotopic abundances are 0.7204 ± 0.0007 atom % and 0.00573 ± 0.00018 atom % for U235 and U234, respectively.