High Precision Linewidth Measurement of Laser-Cooled Atoms: Resolution of the Na3p2P3/2Lifetime Discrepancy

Abstract
We report resolution of the 1% discrepancy between theory and experiment for the lifetime of the first excited state of Na. Determining the atomic lifetime by a novel method, we have measured the natural linewidth of the 32S1/232P3/2 transition with <0.25% accuracy through precision spectroscopy on an optically prepared sample of ultracold, two-level atoms. The resulting 32P3/2 lifetime of 16.237(35) ns disagrees with previous time-domain measurements but is in good agreement with recent calculations and a new fast beam result.