Optical determination of the antiferromagnetic exchange constant between nearest-neighbor Mn2+ ions in Zn0.95Mn0.05Te

Abstract
Zeeman splittings of the free exciton in Zn0.95 Mn0.05Te have been measured at 1.4 K with dc magnetic field B up to 19.3 T, using magnetoreflectance in the Faraday configuration. The splitting between the highest- and lowest-energy Zeeman components of the exciton follows a modified Brillouin function at low values of B≲10 T. The first of the expected five steps due to the magnetic-field-induced alignment of the antiferromagnetically coupled nearest-neighbor (NN) pairs was observed at B1=15.0±0.6 T. Ignoring the effect of internal fields due to distant-neighbor Mn2+ ions on NN pairs, we deduce the NN exchange constant JNN-(1/2)gμB B1=-10. 1±0.4 K, in good agreement with that obtained from magnetization measurements.