Nonadiabatic Alignment of Asymmetric Top Molecules: Field-Free Alignment of Iodobenzene
- 24 July 2003
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 91 (4) , 043003
- https://doi.org/10.1103/physrevlett.91.043003
Abstract
Nonadiabatic laser alignment of an asymmetric top molecule is studied using the combination of a quantum dynamical theory and time-resolved photofragment imaging experiments. In particular, the degree of alignment of iodobenzene, induced by an intense, linearly polarized picosecond laser pulse, is calculated and measured. Pronounced alignment is obtained under field-free conditions.Keywords
This publication has 19 references indexed in Scilit:
- Colloquium: Aligning molecules with strong laser pulsesReviews of Modern Physics, 2003
- On the dynamics of rotationally broad, spatially aligned wave packetsThe Journal of Chemical Physics, 2001
- Three Dimensional Alignment of Molecules Using Elliptically Polarized Laser FieldsPhysical Review Letters, 2000
- Revival Structure of Aligned Rotational Wave PacketsPhysical Review Letters, 1999
- New means of spatially manipulating molecules with lightThe Journal of Chemical Physics, 1999
- Controlling the alignment of neutral molecules by a strong laser fieldThe Journal of Chemical Physics, 1999
- Time evolution of pendular states created by the interaction of molecular polarizability with a pulsed nonresonant laser fieldThe Journal of Chemical Physics, 1999
- Spectroscopy of pendular states in optical-field-aligned speciesThe Journal of Chemical Physics, 1996
- Rotational excitation and molecular alignment in intense laser fieldsThe Journal of Chemical Physics, 1995
- Alignment and Trapping of Molecules in Intense Laser FieldsPhysical Review Letters, 1995