First- and second-chance proton emission in the interactions of fast neutrons withMo92

Abstract
Cross sections were measured radiochemically for the Mo92(n,p)92 Nbm and Mo92(n,n’p +pn+d)91 Nbm reactions over the neutron energy range of 9.010.6 MeV, and for the latter reaction also between 12.6 and 14.4 MeV. Use was made of high-resolution γ-ray and x-ray spectroscopy. Statistical-model calculations taking into account precompound effects were performed for fast neutron induced reactions on Mo92. The calculational results agree well with the experimental data on emitted proton spectra as well as on the excitation functions of various reaction channels. The second-chance proton emission is significant for incident neutron energies above 11 MeV; between 13 and 14 MeV it is comparable to the first-chance proton emission.