Matrix-isolated bismuth. I. The AX band system of Bi2 in solid argon

Abstract
The AX fluorescence system of the Bi2 molecule in solid argon has been explored by means of tunable dye laser radiation. About 135 bands involving A state levels from v′=0 to v′=6 and X state levels up to v′′=26 are observed. Analysis yields ωe values of 133.4 and 174.3 cm−1 for the A and X states, respectively, and a band system origin at 17 719 cm−1. The Raman spectrum of the fundamental vibration and two overtones of Bi2 appear along with the fluorescence.

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