Magnetoreflectivity of Pb1xEuxTe epilayers and PbTe/Pb1xEuxTe multiple quantum wells

Abstract
Molecular-beam epitaxy grown n-type Pb1x EuxTe epilayers (x⩽0.034) and PbTe/Pb1x EuxTe (x⩽0.039) multiple-quantum-well (MQW) samples were studied by magnetoreflectivity in the Faraday configuration (B‖[111]) for magnetic fields up to 6 T at 4.2 K. Since the IV-VI lead salt compounds are quite polar semiconductors, resonant electron-longitudinal-optic- (LO-) phonon coupling (Fröhlich coupling) modifies the cyclotron resonance (CR) energies in the Pb1x EuxTe single epilayers for the three-dimensional (3D) case. Due to the many-valley band structure two different Fröhlich coupling constants are relevant. However, the CR energies of quasi-two-dimensional (2D) carriers in PbTe wells [n2D=(1.5-3)×1011 cm2] of PbTe/Pb1x EuxTe MQW samples do not exhibit a significant resonant electron-LO-phonon interaction. This observation is attributed to finite-electron concentration effects, in particular, to a partial filling of the lowest 2D Landau spin level. The static and dynamic screening of the polar interaction are considered as well, but are ruled out as an explanation for the absence of any remarkable polaron correction to the CR energies of electrons in the PbTe quantum wells for the range of carrier concentrations investigated. The magnetoreflectivity spectra of Pb1x EuxTe single layers and PbTe/Pb1x EuxTe quantum well samples are simulated numerically, using a model for the dielectric response of IV-VI compounds in a magnetic field, which also includes the electron-LO-phonon interaction. The transverse and longitudinal masses, and thus also the interband momentum matrix elements are determined for Pb1x EuxTe as a function of the composition up to x<0.034. It is found that the transverse mass increases with Eu content, whereas the longitudinal one nearly stays constant. The 2D CR masses of electrons in the PbTe wells increase with decreasing well width, i.e., with increasing quantum-well interband energies, a behavior which results from the strong band nonparabolicity.