Fission-evaporation competition in Pu isotopes of mass 235-239

Abstract
Cross sections are reported for the reactions U233,234,235(He4,xn), for x=14. Comparisons are shown to calculations based on equilibrium and preequilibrium models. Fits of preequilibrium-model calculations to the tails of the excitation functions require significantly different parameters from those in the literature for other systems. There is a suggestion for emission of a second preequilibrium neutron. The equilibrium-model calculations show systematic deviations from the data that can be related to the empirically determined energy dependence of Γn(Γn+Γf). The fission barrier parameters for isotopes of Pu are refined. Their relationship to the excitation functions for ground state and shape isomeric nuclei is discussed.