Ferromagnetic Clusters and Magnetic Polarons as Evidenced by ESR in La1.35Sr1.65Mn2O7

Abstract
La1.35Sr1.65Mn2O7 is investigated in the regime where 3D magnetic order is lost but 2D correlations are strong. ESR shows that the localized t2g spins are coupled into intralayer ferromagnetic clusters of fixed size. The eg carriers form polarons with an effective spin growing from 1/2 to 7. ESR and transport properties suggest that the 3D order originates from the onset of coherence of the ferromagnetic clusters mediated by the propagation of the polarons.