Abstract
The stopping power and the range of He++ ions with energies between about 1 and 9 MeV have been measured for the oxides of nuclear interest UO2, and (U, Pu)O2, and ThO2, using a new and versatile method. The experimental technique consisted in evaporating oxide layers onto a source emitting α particles of five different energies, and then determining dEdx by α spectroscopy. These multienergy sources could conveniently be obtained by exposing a metal foil to the recoil atoms of Th228, the radioactive decay chain of which contains five daughter nuclides with different α energies. In addition, the α spectra of thick homogeneous samples were also evaluated and yieldd confirmatory results. The data are compared to theoretical calculations. and their application in self-diffusion studies is discussed.