γemission from the 31-yr isomer of178Hfinduced by x-ray irradiation

Abstract
A sample containing 6.3×1014 nuclei of the 16+ isomer of 178Hf having a half life of 31 years and excitation energy of 2.446 MeV was irradiated with x-ray pulses derived from a device operated at 15 mA to produce bremsstrahlung radiation with an end point energy set to be 63 keV. Gamma spectra of the isomeric target were taken with two independent Ge detectors. Intensities of the 213.4 keV (4+2+) and 325.5 keV (6+4+) transitions in the ground state band of 178Hf were found to increase when irradiated. The largest enhancement was 1.6±0.3% measured in the 213.4 keV transition. Such an accelerated decay of the 178Hf isomer is consistent with an integrated cross section exceeding 2.2×1022cm2keV if the resonant absorption takes place below 20 keV as indicated by the use of selective absorption filters in the irradiating beam.