Stimulated emission and optical gain in a single MOVPE-grown ZnxCd1xSeZnSe quantum well

Abstract
We have studied the stimulated emission from an optically pumped graded index separate confinement heterostructure, realized in the form of a metal-organic vapor-phase-epitaxy-grown single quantum well based on a wide-gap (ZnCd)Se semiconductor. The structure is composed of a central Zn0.78Cd0.22Se quantum well sandwiched between two thicker, zinc-rich (ZnCd)Se layers with a graded cadmium composition varying continuously and monotonously between 0% and 5%. The stimulated emission occurred at 2.49eV (T=8.5K), being spectrally redshifted with increasing temperature and disappearing for T>~200K. The optical gain has been measured using the variable stripe-length method, and values of the gain up to 620cm1 have been achieved. High-resolution spectral studies of the stimulated emission have revealed a fine structure in the emission spectra originating from different localization sites for excitons. We identify the lasing mechanism as due to an inhomogeneously broadened system of localized excitons.