Photoelectron diffraction determination of the geometry of a clean metal surface: Ta(100)

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Abstract
The ratio of photoemission intensities from the bulk- and surface-shifted 4f core levels of the clean Ta(100) surface was measured in two different modes: as a function of photon energy at normal emission and as a function of polar angle near the [011] azimuth at ħω=65 eV. We have also performed a multiple-scattering photoemission calculation for several first interlayer spacings ranging from the bulk value to a 15% contraction. The best agreement with experiment was obtained for a (10±5)% contraction of the first interlayer spacing.