Abstract
High-field magnetization steps due to energy-level crossings for pairs of nearest-neighbor Mn spins were observed in Cd1x MnxS, Cd1x MnxTe, and Zn1x MnxSe. For Cd1x MnxTe, two steps were observed. The difference H2-H1 between the magnetic fields at the centers of these steps gives JNN/kB=6.1±0.3 K for the exchange constant between nearest-neighbor Mn spins. For Cd1x MnxS and Zn1x MnxSe, only the first step at H1 was observed. The values of H1 give the estimates JNN/kB10.5 K for Cd1x MnxS, and JNN/kB12.6 K for Zn1x MnxSe. Our results for JNN in the three materials are in good agreement with other recent determinations. The magnitudes of the magnetization steps in all three materials are consistent with those expected from a random distribution of Mn ions over the cation sites in the crystals.