Time-resolved Photoluminescence and Carrier Dynamics in Vertically-coupled Self-assembled Quantum Dots

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Abstract
The relaxation mechanisms of an array of 10 vertically coupled layers of InGaAs/AlGaAs quantum dots were studied by time-resolved photoluminescence. Both resonant and non-resonant excitation were employed and the photoluminescence (PL) intensity in the non-resonant case is a factor of 200 larger than the intensity with resonant excitation. The results obtained in the non-resonant pumping experiment were analysed with a rate equation model. It was found that the PL decay time increases rapidly with the wavelength of detection. Large carrier capture cross-sections [(2.5±0.9)×10-5 cm3/s] were deduced, resulting in a capture time of 1 ps for a carrier concentration of 4×1016 cm-3. A very fast PL risetime was observed with resonant pumping, ruling out a phonon bottleneck effect in these samples. The decay times at a given wavelength are always shorter for resonant than for non-resonant excitation and their difference increases rapidly with wavelength. This is interpreted in terms of a state filling effect for the non-resonant case.