Light-induced changes of phosphorus bonding configurations in hydrogenated amorphous silicon

Abstract
We report the direct observation of a metastable substitutional phosphorus state in hydrogenated amorphous silicon by nuclear-magnetic-resonance spectroscopy. The fourfold site is identified from the spectra's characteristic chemical shift. The substitutional site is removed by "light-soaking" the film and created by low-temperature annealing. Phosphorus relaxation-time measurements indicate Raman processes dominate the spin-lattice relaxation of the phosphorus nuclei.

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